Design and Synthesis of Multifunctional Metal Organic Materials Systematic Study on Magnetic and Catalytic Properties

Abstract

The design and synthesis of multifunctional metal-organic materials have gained significant attention in recent years due to their unique combination of magnetic and electrocatalytic properties. This systematic study focuses on exploring the correlation between the structural characteristics and the resulting magnetic and electrocatalytic behavior of these materials. Based on this, we have synthesized a 3D Coordination Polymer. Hirshfeld surface analysis indicates the presence of strong hydrogen bonding interactions between the protonated pyridyl Nitrogen atoms and the oxygen atoms of the ligand within compound 1. The magnetic measurements show that compound 1 presents a weak antiferromagnetic coupling with a canted antiferromagnetic long-range order below 14 K with a coercive field of 40 mT at 2 K. In another work two hydrolytically stable Co-pdc MOFs of different dimensionality have been synthesized to study the correlation between dimensionality with electrocatalytic water oxidation behaviour.